Aircraft Emissions’ Contributions to Organic Aerosols in a Regional Air Quality Model using the Volatility Basis Set

نویسندگان

  • Matthew Woody
  • Saravanan Arunachalam
چکیده

A framework that employs the Volatility Basis Set (VBS) within the Community Multiscale Air Quality Model (CMAQ) was applied to predict organic aerosol concentrations from aircraft emissions. This framework was further expanded to include the formation of secondary organic aerosols from semi and intermediate volatile organic compounds which are traditionally missing from emission inventories used in air quality models. Results indicated that CMAQ with VBS predicted similar total contributions to fine particulate matter compared to CMAQ without VBS but with variations in the composition of organic species.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Modeling organic aerosols in a megacity: comparison of simple and complex representations of the volatility basis set approach

The Weather Research and Forecasting model coupled with chemistry (WRF-Chem) is modified to include a volatility basis set (VBS) treatment of secondary organic aerosol formation. The VBS approach, coupled with SAPRC-99 gas-phase chemistry mechanism, is used to model gas-particle partitioning and multiple generations of gas-phase oxidation of organic vapors. In addition to the detailed 9-species...

متن کامل

Modelling of organic aerosols over Europe (2002–2007) using a volatility basis set (VBS) framework: application of different assumptions regarding the formation of secondary organic aerosol

A new organic aerosol module has been implemented into the EMEP chemical transport model. Four different volatility basis set (VBS) schemes have been tested in long-term simulations for Europe, covering the six years 2002–2007. Different assumptions regarding partitioning of primary organic aerosol and aging of primary semi-volatile and intermediate volatility organic carbon (S/IVOC) species an...

متن کامل

Impact of Mexico City emissions on regional air quality from MOZART-4 simulations

An extensive set of measurements was made in and around Mexico City as part of the MILAGRO (Megacity Initiative: Local and Global Research Observations) experiments in March 2006. Simulations with the Model for Ozone and Related Chemical Tracers, version 4 (MOZART4), a global chemical transport model, have been used to provide a regional context for these observations and assist in their interp...

متن کامل

Non-linear partitioning and organic volatility distributions of urban aerosols.

Gas-to-particle partitioning of organic aerosols (OA) is represented in most models by Raoult's law, and depends on the existing mass of particles into which organic gases can dissolve. This raises the possibility of non-linear response of particle-phase OA mass to the emissions of precursor volatile organic compounds (VOCs) that contribute to this partitioning mass. Implications for air qualit...

متن کامل

Online measurements of the emissions of intermediate- volatility and semi-volatile organic compounds from aircraft

A detailed understanding of the climate and air quality impacts of aviation requires measurements of the emissions of intermediate-volatility and semi-volatile organic compounds (I/SVOCs) from aircraft. Currently both the amount and chemical composition of aircraft I/SVOC emissions remain poorly characterized. Here we characterize I/SVOC emissions from aircraft, using a novel instrument for the...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2012